- Abstract:
-
Standard continuum theory fails to predict several key experimental results of electrostatic and electrokinetic measurements at aqueous electrolyte interfaces. In order to extend the continuum theory to include the effects of molecular solvent structure, we generalize the equations for electrokinetic transport to incorporate a space dependent dielectric profile, viscosity profile, and non-electrostatic interaction potential. All necessary profiles are extracted from atomistic molecular dynami...
Expand abstract - Publisher copy:
- 10.1021/jp402482q
-
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- Journal:
- The journal of physical chemistry. B
- Volume:
- 117
- Issue:
- 39
- Pages:
- 11397-11413
- Publication date:
- 2013-10-05
- DOI:
- EISSN:
-
1520-5207
- ISSN:
-
1520-6106
- URN:
-
uuid:a6a58902-7cb6-48ef-9f26-38efe007cf99
- Source identifiers:
-
434465
- Local pid:
- pubs:434465
- Copyright date:
- 2013
Journal article
Beyond the continuum: how molecular solvent structure affects electrostatics and hydrodynamics at solid-electrolyte interfaces.
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