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Thesis

Total synthesis and stereochemical reassignment of dehydromicrosclerodermin B and microsclerodermin J

Abstract:

This thesis describes research towards the total synthesis of two marine natural products, dehydromicrosclerodermin B and microsclerodermin J. The synthesis of the most complex subunit of these peptides, AMMTD, was accomplished in a longest linear sequence of 21 steps starting from (S)-Roche ester. Preliminary results conducted by other group members were improved; the key cuprate displacement reaction and the final steps of the synthetic sequence were developed. Subsequently, AMMTD-GABOB ...

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Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author

Contributors

Role:
Supervisor
Type of award:
DPhil
Level of award:
Doctoral
Awarding institution:
University of Oxford
UUID:
uuid:a0894f3b-0209-4feb-957e-9c4b0bdb60a8
Deposit date:
2017-02-26

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