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Colloidal Cu/ZnO catalysts for the hydrogenation of carbon dioxide to methanol: investigating catalyst preparation and ligand effects

Abstract:

The production of methanol from CO 2 hydrogenation is a promising potential route to a renewable liquid fuel and renewable energy vector. Herein, three distinct routes to make colloidal catalysts based on mixtures of Cu(0) and ZnO nanoparticles (NPs) and using low-temperature organometallic procedures are reported. The colloids are surface coordinated by a phosphinate ligand: dioctylphosphinate ([DOPA] - ), which delivers a high solubility in organic solvents. Further, the synthetic routes a...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Publisher's version

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Publisher copy:
10.1039/C7CY01191A

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Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
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Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
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Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Catalysis Science & Technology Journal website
Volume:
7
Issue:
17
Pages:
3842-3850
Publication date:
2017-08-11
Acceptance date:
2017-07-26
DOI:
EISSN:
2044-4761
ISSN:
2044-4753
Pubs id:
pubs:729100
URN:
uri:9f38d42f-3c6c-41b2-a38c-d784edb3f778
UUID:
uuid:9f38d42f-3c6c-41b2-a38c-d784edb3f778
Local pid:
pubs:729100
Keywords:

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