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Cage occupancy and compressibility of deuterated N-2-clathrate hydrate by neutron diffraction

Abstract:

This paper reports pressure dependent high resolution neutron diffraction work on N2-clathrates, which for the first time provides numbers on the compressibility as well as the location and degree of filling of the guest molecules in the small and large cages. N2-clathrates crystallize, at least at lower pressures and temperatures near 0 °C, in the Stackelberg type II structure. However, during the diffraction experiments we have observed the transient and partial formation of the von Stackel...

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Publication status:
Published

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Publisher copy:
10.1023/A:1007960217691

Authors


Chazallon, B More by this author
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Institution:
University of Oxford
Department:
Oxford, MPLS, Physics, Condensed Matter Physics
Journal:
JOURNAL OF INCLUSION PHENOMENA AND MOLECULAR RECOGNITION IN CHEMISTRY
Volume:
29
Issue:
1
Pages:
65-77
Publication date:
1997-09-05
DOI:
ISSN:
0923-0750
URN:
uuid:9bfd5643-8e6f-49b0-bd96-bf1d091461f0
Source identifiers:
66389
Local pid:
pubs:66389

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