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Structural snapshots of concerted double E–H bond activation at a transition metal centre

Abstract:

Bond activation at a transition metal centre is a key fundamental step in numerous chemical transformations. The oxidative addition of element–hydrogen bonds, for example, represents a critical step in a range of widely applied catalytic processes. Despite this, experimental studies defining steps along the bond activation pathway are very rare. In this work, we report on fundamental studies defining a new oxidative activation pathway: combined experimental and computational approaches yield ...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted manuscript

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Publisher copy:
10.1038/nchem.2792

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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
Role:
Author
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Publisher:
Springer Nature Publisher's website
Journal:
Nature Chemistry Journal website
Volume:
9
Pages:
1256–1262
Publication date:
2017-06-12
Acceptance date:
2017-05-04
DOI:
EISSN:
1755-4349
ISSN:
1755-4330
Pubs id:
pubs:714186
URN:
uri:9bcdf1f9-72e7-454e-9060-08f6ebec59f3
UUID:
uuid:9bcdf1f9-72e7-454e-9060-08f6ebec59f3
Local pid:
pubs:714186

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