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Influence of dipolar interactions on radical pair recombination reactions subject to weak magnetic fields.

Abstract:

Monte Carlo simulations of the effects of weak magnetic fields on the recombination of interacting radical pairs undergoing free diffusion in solution have been performed, with the aim of determining the influence on the low field effect of the magnetic dipolar coupling between the radicals. The suppression of singlet-triplet interconversion in the radical pair by the dipolar interaction is found to be pronounced at magnetic field strengths comparable to the hyperfine interactions in the radi...

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Publication status:
Published

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Publisher copy:
10.1021/jp0456943

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
Journal:
journal of physical chemistry. A More from this journal
Volume:
109
Issue:
5
Pages:
869-873
Publication date:
2005-02-01
DOI:
EISSN:
1520-5215
ISSN:
1089-5639
Language:
English
Keywords:
Pubs id:
pubs:33543
UUID:
uuid:8e423be3-f7e9-4682-b50d-182b6382e90e
Local pid:
pubs:33543
Source identifiers:
33543
Deposit date:
2012-12-19

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