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Cyclic Voltammetry of the EC' Mechanism at Hemispherical Particles and Their Arrays: The Split Wave

Abstract:

The EC′ (catalytic) mechanism, (1) A + e- ⇌ B; (2) B + X → K2 A + P, in which the reduction of X to P is mediated by the A/B redox couple, is studied at a regularly distributed array of hemispherical particles on a planar surface using simulated cyclic voltammetry. It is assumed that the supporting surface itself is not electroactive and therefore the electron transfer in process (1) occurs exclusively on the surface of the particles. Two-dimensional finite difference simulations are performe...

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Publication status:
Published

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Publisher copy:
10.1021/jp2023204

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
Journal:
JOURNAL OF PHYSICAL CHEMISTRY C
Volume:
115
Issue:
22
Pages:
11204-11215
Publication date:
2011-06-09
DOI:
EISSN:
1932-7455
ISSN:
1932-7447
Language:
English
Pubs id:
pubs:159287
UUID:
uuid:8e196134-8694-4652-ac72-8a8c725c615b
Local pid:
pubs:159287
Source identifiers:
159287
Deposit date:
2012-12-19

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