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Tracking thermal-induced amorphization of a zeolitic imidazolate framework via synchrotron in situ far-infrared spectroscopy.

Abstract:
We present the first use of in situ far-infrared spectroscopy to analyze the thermal amorphization of a zeolitic imidazolate framework material. We explain the nature of vibrational motion changes during the amorphization process and reveal new insights into the effect that temperature has on the Zn-N tetrahedra.
Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted manuscript

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Publisher copy:
10.1039/c7cc01985h

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Department:
Oxford, MPLS, Engineering Science
Role:
Author
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Royal Society More from this funder
Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Chemical Communications Journal website
Volume:
53
Issue:
52
Pages:
7041-7044
Publication date:
2017-06-06
Acceptance date:
2017-06-06
DOI:
EISSN:
1364-548X
ISSN:
1359-7345
Pubs id:
pubs:700716
URN:
uri:8c45f1c3-a119-4422-8e1b-ac127e8c55e9
UUID:
uuid:8c45f1c3-a119-4422-8e1b-ac127e8c55e9
Local pid:
pubs:700716
Language:
English
Keywords:

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