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Impacts reveal and quantify monolayer adsorption on single alumina particles

Abstract:

A particle impact method is used to quantify adsorption of redox active species on single insulating particles by simulation of individual spike transient, circumventing the complexity of measurements with ensembles of particles. For catechol, anthraquinone and chloranil molecules and the ferrocene moiety of poly(vinylferrocene) adsorbed on alumina, the surface coverages are found to be (3.0 ± 0.9), (1.5 ± 1.4), (2.7 ± 1.7) and (2.1 ± 0.7) × 10–10 mol cm–2, and the charge diffusion coefficien...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted Manuscript

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Publisher copy:
10.1134/S1023193517090087

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Department:
Oxford, MPLS, Chemistry, Physical & Theoretical Chem
Role:
Author
More by this author
Department:
Oxford, MPLS, Chemistry, Physical & Theoretical Chem
Role:
Author
Publisher:
Pleiades Publishing Publisher's website
Journal:
Russian Journal of Electrochemistry Journal website
Volume:
53
Issue:
9
Pages:
994–1002
Publication date:
2017-09-23
Acceptance date:
2016-11-15
DOI:
EISSN:
1608-3342
ISSN:
1023-1935
Pubs id:
pubs:664981
URN:
uri:8abae019-d101-4672-83e4-709ee66b2a66
UUID:
uuid:8abae019-d101-4672-83e4-709ee66b2a66
Local pid:
pubs:664981
Paper number:
9

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