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Capacity-limiting mechanisms in Li/O2 batteries.

Abstract:

A continuum model of an aprotic lithium/oxygen battery is validated against experimental first-discharge data and used to examine how the apparent cell capacity is affected by macroscopic multicomponent mass transfer, interfacial kinetics, and electronic conduction or tunneling through the discharge product. The model accounts for the three-phase nature of the positive electrode in detail, including an explicit discharge-product layer whose properties and volume distribution generally depend ...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Publisher's version

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Publisher copy:
10.1039/c6cp04055a

Authors


Rahimian, SK More by this author
More by this author
Department:
St Peters College
Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Physical Chemistry Chemical Physics Journal website
Volume:
18
Pages:
22840-22851
Publication date:
2016-07-05
Acceptance date:
2016-07-01
DOI:
ISSN:
1463-9084
Pubs id:
pubs:636394
URN:
uri:7e69f47d-a0c5-454a-948b-afead46336b8
UUID:
7e69f47d-a0c5-454a-948b-afead46336b8
Local pid:
pubs:636394
Language:
English
Keywords:

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