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The Subtleties of the Reversible Hydrogen Evolution Reaction Arising from the Nonunity Stoichiometry

Abstract:

© 2015 American Chemical Society. The proton/hydrogen redox couple underpins the electrochemical sciences; however, the nonunity stoichiometry of the reaction leads to distinct voltammetric complications. This Article provides a joint analytical, numerical, and experimental investigation into the reversible hydrogen evolution reaction at a platinum microelectrode. Literature obscurities and nuances are highlighted and corrected, allowing the presentation of an holistic overview of the electro...

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Publication status:
Published
Peer review status:
Peer Reviewed

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Publisher copy:
10.1021/acs.jpcc.5b01864

Authors


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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Role:
Author
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Grant:
FP/2007-2013/ ERC Grant No. 320403
Journal:
Journal of Physical Chemistry C
Volume:
119
Issue:
17
Pages:
9402-9410
Publication date:
2015-04-30
DOI:
EISSN:
1932-7455
ISSN:
1932-7447
URN:
uuid:7929dd60-6945-4261-b860-5d3206d686ca
Source identifiers:
524410
Local pid:
pubs:524410

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