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Photodissociation dynamics of OCS at 248nm: the S(¹D2) atomic angular momentum polarization

Abstract:

The dissociation of OCS has been investigated subsequent to excitation at 248 nm. Speed distributions, speed dependent translational anisotropy parameters, angular momentum alignment, and orientation are reported for the channel leading to S(¹D2). In agreement with previous experiments, two product speed regimes have been identified, correlating with differing degrees of rotational excitation in the CO coproducts. The velocity dependence of the translational anisotropy is also shown to be in ...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Publisher's version

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Publisher copy:
10.1063/1.2757618

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Institution:
University of Oxford
Research group:
Brouard Group: Gas Phase Reaction Dynamics
Department:
Mathematical,Physical & Life Sciences Division - Chemistry - Physical and Theoretical Chemistry Laboratory
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Mathematical,Physical & Life Sciences Division - Chemistry - Physical and Theoretical Chemistry Laboratory
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Mathematical,Physical & Life Sciences Division - Chemistry - Physical and Theoretical Chemistry Laboratory
Role:
Author
More by this author
Institution:
University of Oxford
Research group:
Vallance Group
Department:
Mathematical,Physical & Life Sciences Division - Chemistry - Physical and Theoretical Chemistry Laboratory
Role:
Author
Engineering and Physical Sciences Research Council More from this funder
Publisher:
American Institute of Physics Publisher's website
Journal:
Journal of Chemical Physics Journal website
Volume:
127
Issue:
8
Pages:
Article: 084304
Publication date:
2007-08-05
DOI:
EISSN:
1089-7690
ISSN:
0021-9606
URN:
uuid:74d9230d-1525-438b-8574-5543fd367ab9
Local pid:
ora:1736

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