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Photodissociation dynamics of OCS at 248nm: the S(¹D2) atomic angular momentum polarization

Abstract:

The dissociation of OCS has been investigated subsequent to excitation at 248 nm. Speed distributions, speed dependent translational anisotropy parameters, angular momentum alignment, and orientation are reported for the channel leading to S(¹D2). In agreement with previous experiments, two product speed regimes have been identified, correlating with differing degrees of rotational excitation in the CO coproducts. The velocity dependence of the translational anisotropy is also shown to be in ...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1063/1.2757618

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Research group:
Brouard Group: Gas Phase Reaction Dynamics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Research group:
Vallance Group
Role:
Author
Engineering and Physical Sciences Research Council More from this funder
Publisher:
American Institute of Physics Publisher's website
Journal:
Journal of Chemical Physics Journal website
Volume:
127
Issue:
8
Article number:
084304
Publication date:
2007-08-01
DOI:
EISSN:
1089-7690
ISSN:
0021-9606
Language:
English
Keywords:
Subjects:
UUID:
uuid:74d9230d-1525-438b-8574-5543fd367ab9
Local pid:
ora:1736
Deposit date:
2008-03-14

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