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Quantitative analysis of valence photoemission spectra and quasiparticle excitations at chromophore-semiconductor interfaces.

Abstract:

Investigating quasiparticle excitations of molecules on surfaces through photoemission spectroscopy forms a major part of nanotechnology research. Resolving spectral features at these interfaces requires a comprehensive theory of electron removal and addition processes in molecules and solids which captures the complex interplay of image charges, thermal effects, and configurational disorder. Here, we develop such a theory and calculate the quasiparticle energy-level alignment and the valence...

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Publication status:
Published

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Authors


Patrick, CE More by this author
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Institution:
University of Oxford
Department:
Oxford, MPLS, Materials
Journal:
Physical review letters
Volume:
109
Issue:
11
Pages:
116801
Publication date:
2012-09-05
DOI:
EISSN:
1079-7114
ISSN:
0031-9007
URN:
uuid:74b2aa61-b2cf-43ce-b815-b3cddd9f63cd
Source identifiers:
352501
Local pid:
pubs:352501

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