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Quantifying the Exchange Coupling in Linear Copper Porphyrin Oligomers

Abstract:

Linear π-conjugated porphyrin oligomers are of significant current interest due to their potential applications as molecular wires. In this study we investigate electronic communication in linear butadiyne-linked copper porphyrin oligomers by electron paramagnetic resonance (EPR) spectroscopy via measurement of the exchange interaction, J, between the copper(II) centers. The contributions of dipolar and exchange interactions to the frozen solution continuous wave (cw) EPR spectr...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Publisher's version

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Publisher copy:
10.1039/C7CP01787A

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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry
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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry
Suturina, E More by this author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry
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Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Physical Chemistry Chemical Physics Journal website
Volume:
19
Issue:
24
Pages:
16057
Publication date:
2017-06-09
Acceptance date:
2017-05-29
DOI:
ISSN:
1463-9084
Pubs id:
pubs:698725
URN:
uri:71e77567-ed4d-4545-b7ef-e33e8bf1a54c
UUID:
uuid:71e77567-ed4d-4545-b7ef-e33e8bf1a54c
Local pid:
pubs:698725

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