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Thermal convection in electrochemical cells. Boundaries with heterogeneous thermal conductivity and implications for scanning electrochemical microscopy

Abstract:

We investigate the heat transfer in a cylinder-shaped electrochemical cell with solid, thermally insulating walls. The cell is filled with a liquid and a solid substrate that is thermostated from below is situated at its base. The initial temperature of the liquid is different from that of the substrate so as to mimic imperfect thermostating in an electrochemical experiment; as heat transfer acts to diminish the temperature difference between the two, natural convection ensues. The influence ...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted manuscript

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Publisher copy:
10.1039/C7CP01797A

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Department:
Oxford, MPLS, Chemistry, Physical & Theoretical Chem
Role:
Author
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Department:
Oxford, MPLS, Chemistry, Physical & Theoretical Chem
Role:
Author
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Funding agency for:
Novev, JK
Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Physical Chemistry Chemical Physics Journal website
Volume:
19
Issue:
20
Pages:
12759-12775
Publication date:
2017-05-04
Acceptance date:
2017-05-04
DOI:
EISSN:
1463-9084
ISSN:
1463-9076
Pubs id:
pubs:692433
URN:
uri:705e9203-969a-47b8-907f-6d16a51740f2
UUID:
uuid:705e9203-969a-47b8-907f-6d16a51740f2
Local pid:
pubs:692433

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