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Nanoparticle-electrode collision processes: Investigating the contact time required for the diffusion-controlled monolayer underpotential deposition on impacting nanoparticles

Abstract:

Recent work on faradaic processes occurring during thermal nanoparticle-electrode collisions contrasts significantly from analogous research using ultrasonically-driven microparticles, where no faradaic signals were found. It is suggested that this might be explained by the differences in both particle size and contact time. To investigate this, we present results from adapted Monte Carlo random walk simulations. Using the underpotential deposition of thallium onto silver nanoparticles as a m...

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Publication status:
Published

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
Journal:
CHEMICAL PHYSICS LETTERS More from this journal
Volume:
514
Issue:
1-3
Pages:
58-61
Publication date:
2011-09-27
DOI:
ISSN:
0009-2614
Language:
English
UUID:
uuid:6d920090-70e9-4eca-a355-a9e29b373f38
Local pid:
pubs:179960
Source identifiers:
179960
Deposit date:
2012-12-19

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