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Extending electron orbital precession to the molecular case: Use of orbital alignment for observation of wavepacket dynamics

Abstract:

The complexity of ultrafast molecular photoionization presents an obstacle to the modeling of pump-probe experiments. Here, a simple optimized model of atomic rubidium is combined with a molecular dynamics model to predict quantitatively the results of a pump-probe experiment in which long-range rubidium dimers are first excited, then ionized after a variable delay. The method is illustrated by the outline of two proposed feasible experiments and the calculation of their outcomes. Both of the...

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Publication status:
Published

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Publisher copy:
10.1103/PhysRevA.83.043419

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Institution:
University of Oxford
Department:
Oxford, MPLS, Physics, Atomic and Laser Physics
Role:
Author
Journal:
PHYSICAL REVIEW A
Volume:
83
Issue:
4
Publication date:
2011-04-29
DOI:
EISSN:
1094-1622
ISSN:
1050-2947
URN:
uuid:6cf1f122-8c7a-4efe-8e09-b223e388897c
Source identifiers:
146616
Local pid:
pubs:146616
Language:
English

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