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Cu/M:ZnO (M = Mg, Al, Cu) colloidal nanocatalysts for the solution hydrogenation of carbon dioxide to methanol

Abstract:

Doped-ZnO nanoparticles, capped with dioctylphosphinate ligands, are synthesised by the controlled hydrolysis of a mixture of organometallic precursors. Substitutional doping of the wurtzite ZnO nanoparticles with 5 mol% Mg(II), Al(III) and Cu(I) is achieved by the addition of sub-stoichiometric amounts of the appropriate dopant [(n-butyl)(sec-butyl)magnesium, triethylaluminium or mesitylcopper] to diethylzinc in the precursor mixture. After hydrolysis, the resulting colloidal nanoparticles (...

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Publication status:
Published
Peer review status:
Peer reviewed

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Files:
Publisher copy:
10.1039/d0ta00509f

Authors


Publisher:
Royal Society of Chemistry
Journal:
Journal of Materials Chemistry A More from this journal
Volume:
8
Issue:
22
Pages:
11282-11291
Publication date:
2020-05-27
Acceptance date:
2020-05-15
DOI:
EISSN:
2050-7496
ISSN:
2050-7488
Language:
English
Keywords:
Pubs id:
1113129
Local pid:
pubs:1113129
Deposit date:
2020-06-26

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