- Abstract:
-
We present a new method for calculating the product yield of a radical pair recombination reaction in the presence of a weak time-dependent magnetic field. This method successfully circumvents the computational difficulties presented by a direct solution of the Liouville-von Neumann equation for a long-lived radical pair containing many hyperfine-coupled nuclear spins. Using a modified formulation of Floquet theory, treating the time-dependent magnetic field as a perturbation, and exploiting ...
Expand abstract - Publication status:
- Published
- Peer review status:
- Peer reviewed
- Version:
- Accepted manuscript
- Files:
-
-
(pdf, 483.7KB)
-
- Publisher copy:
- 10.1063/1.4963793
-
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- Grant:
- FP7/2007-2013/ERC Grant Agreement No. 340451
- Publisher:
- AIP Publishing Publisher's website
- Journal:
- Journal of Chemical Physics Journal website
- Volume:
- 145
- Issue:
- 12
- Chapter number:
- 124117
- Publication date:
- 2016-09-30
- Acceptance date:
- 2016-09-16
- DOI:
- EISSN:
-
1089-7690
- ISSN:
-
0021-9606
- Pubs id:
-
pubs:644373
- URN:
-
uri:670b176f-632b-4891-ac9c-b8ca95299f7f
- UUID:
-
uuid:670b176f-632b-4891-ac9c-b8ca95299f7f
- Local pid:
- pubs:644373
- Paper number:
- 12
- Copyright holder:
- Hiscock et al.
- Copyright date:
- 2016
- Notes:
- Author(s) retain copyright; published by AIP Publishing under license. This is the accepted manuscript version of the article. The final version is available online from AIP at: [10.1063/1.4963793]
Journal article
Floquet theory of radical pairs in radiofrequency magnetic elds
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+ European Research Council
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