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Balanced-detection Raman-induced Kerr-effect spectroscopy

Abstract:

We introduce balanced-detection (BD) Raman-induced Kerr-effect (RIKE) as a powerful coherent Raman scattering (CRS) technique. RIKE relies on the Raman-induced birefringence that occurs when the pump-Stokes frequency detuning is in resonance with a vibrational transition. We show how a balanced-detection configuration, inspired by that applied in electro-optic sampling, suppresses both the linear and nonlinear backgrounds that affect other CRS techniques. BD-RIKE enables homodyne amplificatio...

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Publication status:
Published

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Publisher copy:
10.1103/PhysRevA.86.053810

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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Role:
Author
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Journal:
PHYSICAL REVIEW A
Volume:
86
Issue:
5
Publication date:
2012-11-09
DOI:
EISSN:
1094-1622
ISSN:
1050-2947
URN:
uuid:6611f796-bd0f-429f-b57e-5858db7823bb
Source identifiers:
366424
Local pid:
pubs:366424
Language:
English

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