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Structure and magnetism of (La/Sr)2M0.5IrV0.5O4 and topochemically reduced (La/Sr)2M0.5IrII0.5O3 (M = Fe, Co) complex oxides

Abstract:

Neutron powder diffraction data show that Sr2Fe0.5Ir0.5O4, Sr2Co0.5Ir0.5O4, and La0.5Sr1.5Co0.5Ir0.5O4 all adopt undistorted, n = 1 Ruddlesden-Popper structures in which the Ir5+ and Fe3+/Co3+/Co2+ cations are statistically disordered over all the octahedral coordination sites. Magnetization data indicate the two cobalt phases are spin glasses at low temperature, while Sr2Fe0.5Ir0.5O4 appears to adopt an antiferromagnetic state with very small magnetically ordered domains. Topochemical reduct...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/acs.inorgchem.9b00541

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Oxford college:
Somerville College
Role:
Author
ORCID:
0000-0002-6248-2063
Publisher:
American Chemical Society Publisher's website
Journal:
Inorganic Chemistry Journal website
Volume:
58
Issue:
2019
Pages:
6336-6343
Publication date:
2019-04-18
Acceptance date:
2019-04-08
DOI:
EISSN:
1520-510X
ISSN:
0020-1669
Pmid:
30998321
Language:
English
Keywords:
Pubs id:
pubs:993215
UUID:
uuid:64b3db2d-fd92-4dce-9446-780c07631f49
Local pid:
pubs:993215
Source identifiers:
993215
Deposit date:
2019-04-23

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