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Transfer of spin correlation between radical pairs in the initial steps of photosynthetic energy conversion

Abstract:

A simple theoretical description of the transfer of electron spin-correlation from one radical pair to another is presented. Solution of the coupled equations of motion of the two radical pairs, yields simple expressions for the spinpolarized electron paramagnetic resonance intensities of the secondary pair in terms of the magnetic and exchange interactions of the electron spins, and the rates of the forward and backward electron transfer reactions of the primary pair. This work is set in the...

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Publication status:
Published

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Publisher copy:
10.1080/002689796173598

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
Journal:
MOLECULAR PHYSICS More from this journal
Volume:
89
Issue:
4
Pages:
1195-1202
Publication date:
1996-11-01
DOI:
ISSN:
0026-8976
Language:
English
Pubs id:
pubs:45390
UUID:
uuid:61e4b588-494f-4680-b35f-617c45cf38c1
Local pid:
pubs:45390
Source identifiers:
45390
Deposit date:
2012-12-19

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