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Novel pulse sequences for time-resolved photo-CIDNP

Abstract:

The properties of a new class of pulse sequences for photo-CIDNP (photochemically induced dynamic nuclear polarization) are analysed in detail, and guidelines for their optimization and applicability are derived. Sensitivity is a central problem with time-resolved photo-CIDNP experiments. By using multiple laser flashes per acquisition and storing the polarizations temporarily in the spin system, a significant improvement is achieved. An alternative application is the reduction of the absorbe...

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Publication status:
Published

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Publisher copy:
10.1080/00268970600634431

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
Host title:
MOLECULAR PHYSICS
Volume:
104
Issue:
10-11
Pages:
1675-1686
Publication date:
2006-05-20
DOI:
EISSN:
1362-3028
ISSN:
0026-8976
Source identifiers:
39966
Keywords:
Pubs id:
pubs:39966
UUID:
uuid:52d06c54-781d-47bb-9f12-1433cefa0614
Local pid:
pubs:39966
Deposit date:
2012-12-19

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