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An electrochemical study of the oxidation of hydrogen at platinum electrodes in several room temperature ionic liquids.

Abstract:

The electrochemical oxidation of dissolved hydrogen gas has been studied in a range of room-temperature ionic liquids (RTILs), namely [C(2)mim][NTf(2)], [C(4)mim][NTf(2)], [N(6,2,2,2)][NTf(2)], [P(14,6,6,6)][NTf(2)], [C(4)mpyrr][NTf(2)], [C(4)mim][BF(4)], [C(4)mim][PF(6)], [C(4)mim][OTf], and [C(6)mim]Cl on a platinum microdisk electrode of diameter 10 microm. In all cases, except [C(6)mim]Cl, a broad quasi-electrochemically reversible oxidation peak between 0.3 to 1.3 V vs Ag was seen prior ...

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Publication status:
Published

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Publisher copy:
10.1021/jp067236v

Authors


Silvester, DS More by this author
Hardacre, C More by this author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Journal:
The journal of physical chemistry. B
Volume:
111
Issue:
18
Pages:
5000-5007
Publication date:
2007-05-05
DOI:
EISSN:
1520-5207
ISSN:
1520-6106
URN:
uuid:4ee5afb1-58dd-42f3-b992-7565648f4d4b
Source identifiers:
33749
Local pid:
pubs:33749

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