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Separation of electron-transfer and coupled chemical reaction components of biocatalytic processes using Fourier transform ac voltammetry.

Abstract:

The underlying electron-transfer and coupled chemical processes associated with biologically important catalytic reactions can be resolved using a combination of Fourier transform ac voltammetry with an analysis of the separated dc and ac components. This outcome can be achieved because the response associated with generation of the catalytic current is essentially confined to the steady-state dc component, whereas the electron-transfer step is dominant in the fundamental and higher harmonics...

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Publication status:
Published

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Publisher copy:
10.1021/ac048151y

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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
Role:
Author
Journal:
Analytical chemistry
Volume:
77
Issue:
11
Pages:
3502-3510
Publication date:
2005-06-05
DOI:
EISSN:
1520-6882
ISSN:
0003-2700
URN:
uuid:4a24e9f8-8077-4d29-951c-620602c97721
Source identifiers:
39485
Local pid:
pubs:39485

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