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Resolving vibrational from electronic coherences in two-dimensional electronic spectroscopy: The role of the laser spectrum

Abstract:

The observation of coherent quantum effects in photosynthetic light-harvesting complexes prompted the question whether quantum coherence could be exploited to improve the efficiency in new energy materials. The detailed characterization of coherent effects relies on sensitive methods such as two-dimensional electronic spectroscopy (2D-ES). However, the interpretation of the results produced by 2D-ES is challenging due to the many possible couplings present in complex molecular structures. In ...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted Manuscript

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Authors


Camargo, FVDA More by this author
Grimmelsmann, L More by this author
More by this author
Department:
Oxford, MPLS, Chemistry, Organic Chemistry
Heisler, IA More by this author
Publisher:
American Physical Society Publisher's website
Journal:
Physical Review Letters Journal website
Volume:
118
Issue:
3
Pages:
Article: 033001
Publication date:
2017
Acceptance date:
2016-12-14
DOI:
EISSN:
1079-7114
ISSN:
0031-9007
Pubs id:
pubs:666509
URN:
uri:49eac654-3b63-4605-8932-c146815978ed
UUID:
uuid:49eac654-3b63-4605-8932-c146815978ed
Local pid:
pubs:666509

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