- Abstract:
-
Atomistic models based on quantum-chemical calculations are combined with time-resolved spectroscopic investigations to explore the migration of electronic excitations along oligophenylenevinylene-based chiral stacks. It is found that the usual Pauli master equation (PME) approach relying on uncoherent transport between individual chromophores underestimates the excitation diffusion dynamics, monitored here by the time decay of the transient polarization anisotropy. A better agreement to expe...
Expand abstract - Publication status:
- Published
- Publisher copy:
- 10.1021/jp050792p
-
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- Journal:
- The journal of physical chemistry. B
- Volume:
- 109
- Issue:
- 21
- Pages:
- 10594-10604
- Publication date:
- 2005-06-05
- DOI:
- EISSN:
-
1520-5207
- ISSN:
-
1520-6106
- URN:
-
uuid:4501771b-7a08-4e20-8739-b6a1161f4ca2
- Source identifiers:
-
23953
- Local pid:
- pubs:23953
- Language:
- English
- Copyright date:
- 2005
Journal article
Excitation migration along oligophenylenevinylene-based chiral stacks: delocalization effects on transport dynamics.
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