- Abstract:
-
Since the 1970s, spin-selective reactions of radical pairs have been modelled theoretically by adding phenomenological rate equations to the quantum mechanical equation of motion of the radical pair spin density matrix. Here, using a quantum measurement approach, we derive an alternative set of rate expressions which predict a faster decay of coherent superpositions of the singlet and triplet radical pair states. The difference between the two results, however, is not dramatic and would proba...
Expand abstract - Publication status:
- Published
- Peer review status:
- Peer reviewed
- Publisher copy:
- 10.1016/j.cplett.2010.01.063
-
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- Publisher:
- Elsevier Publisher's website
- Journal:
- Chemical Physics Letters Journal website
- Volume:
- 488
- Issue:
- 1-3
- Pages:
- 90-93
- Publication date:
- 2010-03-05
- DOI:
- ISSN:
-
0009-2614
- URN:
-
uuid:3874f52f-8b8e-485e-9694-f4319e83807f
- Local pid:
- ora:3702
- Language:
- English
- Subjects:
- Copyright holder:
- Elsevier B. V.
- Copyright date:
- 2010
- Notes:
- The full-text of this article is not currently available in ORA, but you may be able to access the article via the publisher copy link on this record page.
Journal article
Spin-selective reactions of radical pairs act as quantum measurements
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