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Synthesis, anion binding studies and applications of mono- and bimetallic lanthanide complexes

Abstract:

This work describes the preparation and study of lanthanide complexes derived from heptadentate DO3A and DO3AM ligands. The work described encompasses a range of synthetic studies using conventional Click chemistry, novel gold catalysed couplings to prepare mono- and bi- metallic complexes and synthesis of DO3AM derivatives. These complexes have been used in a variety of studies to explore proton and anion binding events, and to develop catalysts for fluorination in protic solvents.

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Department:
University of Oxford
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Supervisor
Type of award:
DPhil
Level of award:
Doctoral
Awarding institution:
University of Oxford

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