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Competition between triplet pair formation and excimer-like recombination controls singlet fission yield

Abstract:

The ultimate goal for singlet fission is that each photo-excited singlet exciton, S1, will result in two triplet excitons with unity yield. However, the singlet fission is now recognized to be complicated, involving bright/dark excited states of different spin multiplicity. Identifying the role of such states is vital to optimize singlet fission yield but difficult due to their elusive spectral signature. Here, we develop an experimental protocol based on a refined magneto-optical probe to ac...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1016/j.xcrp.2021.100339

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Role:
Author
ORCID:
0000-0001-7155-7103
Publisher:
Cell Press
Journal:
Cell Reports Physical Science More from this journal
Volume:
2
Issue:
2
Article number:
100339
Publication date:
2021-02-08
Acceptance date:
2021-01-15
DOI:
EISSN:
2666-3864
Language:
English
Keywords:
Pubs id:
1166216
Local pid:
pubs:1166216
Deposit date:
2021-04-16

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