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Chemistry at the nanoscale: synthesis of an N@C60-N@C60 endohedral fullerene dimer.

Abstract:
Rattling the cage: The rapid one-pot double 1,3-dipolar cycloaddition reaction of the rare endohedral fullerene N@C 60 to an oligo(p-phenylene polyethylene) bis(aldehyde) using a novel amino acid derivative as an anchoring group is reported. The method provides the first example of a chemically linked, two-spin-center N@C 60-N@C 60 molecule (see picture). Assessment of this platform as an element of a quantum computing register is attractive. © 2012 Wiley-VCH Verlag GmbH and Co. KGaA, Weinheim.
Publication status:
Published

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Publisher copy:
10.1002/anie.201107490

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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
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Journal:
Angewandte Chemie (International ed. in English)
Volume:
51
Issue:
15
Pages:
3587-3590
Publication date:
2012-04-01
DOI:
EISSN:
1521-3773
ISSN:
1433-7851
Source identifiers:
312999
Language:
English
Keywords:
Pubs id:
pubs:312999
UUID:
uuid:1f26df7c-60eb-44fd-95a9-4bde094886a9
Local pid:
pubs:312999
Deposit date:
2012-12-19

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