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The [4+2], not [2+2], mechanism occurs in the gold-catalyzed intramolecular oxygen transfer reaction of 2-alkynyl-1,5-diketones.

Abstract:
[2+2] or [4+2]? Mechanistic studies on the gold-catalyzed intramolecular oxygen transfer of 2-alkynyl-1,5-diketones were performed using isotopic experiments and quantum chemical calculations. The results demonstrate that the transformation follow...Expand abstract...
Publication status:
Published

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Publisher copy:
10.1002/anie.201005514

Authors


Malhotra, D More by this author
Hammond, GB More by this author
Journal:
Angewandte Chemie (International ed. in English) More in this journal
Volume:
49
Issue:
48
Pages:
9132-9135
Publication date:
2010-11-19
DOI:
EISSN:
1521-3773
ISSN:
1433-7851
URN:
uuid:426b0814-322a-471a-a7e6-da3754664ad4
Source identifiers:
117661
Local pid:
pubs:117661

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